[CPMD-list] doubt of titanium Ti pseudopotential

Eduardo Ariel Menendez P emenendez at macul.ciencias.uchile.cl
Thu Sep 23 03:34:35 CEST 2004


Hello,

I have the following two doubts. The follwing input and output refers
to a calculation of Ti_6Si_2C_4. I use a supplied pseudopotential that has
the valence shell 3s2 3p6 4s2 3d2. This makes a total of 10 electrons per
Ti. Considering 4 electrons per Si and C, I have a total of
6*10+4*2+4*4=84 electrons
However, looking at the section OCCUPATION I count 48 states. Looking at
the section of basis sets one can see
 GENERATE ATOMIC BASIS SET
 Ti        SLATER ORBITALS
   3D        ALPHA=   3.8833      OCCUPATION= 2.00
   4S        ALPHA=   0.8514      OCCUPATION= 2.00
It seems that the 3p orbitals are ignored. The occupation of 48 states is
consistent with this.

My second dounbt is related to the fact that the Ti pseudopotential has
a proyector for level 4F. The manual of CPMD states that LMAX can be
S,P,or D. However, the CPMD accepts F without complain. The output seems
as
it is understood
 ****************************************************************
 *   ATOM       MASS   RAGGIO NLCC              PSEUDOPOTENTIAL *
 *     Ti    47.9000   1.2000  YES    KLEINMAN      S  NONLOCAL *
 *                                                  P     LOCAL *
 *                                                  D  NONLOCAL *
 *                                                  F  NONLOCAL *
Is this effective?

Thanks
Eduardo

Follows INPUT and partial output.

&CPMD
  OPTIMIZE WAVEFUNCTION
MAXSTEP
1000
STRUCTURE BONDS ANGLES
&END

&DFT
NEWCODE
&END

&SYSTEM
  SYMMETRY
    4
  CHECK SYMMETRY OFF
  CELL DEGREE
     3.0575 1.0  5.764022   90.0 90.0 120.0
  CUTOFF
    80.0
  ANGSTROM
  SCALE
KPOINTS SCALED
 15
  0.0000000  0.0000000  0.0000000   1.00
  0.2000000  0.1154701  0.0000000   6.00
  0.4000000  0.2309401  0.0000000   6.00
  0.2000000  0.3464102  0.0000000   6.00
  0.4000000  0.4618802  0.0000000   6.00
  0.0000000  0.0000000  0.0346980   2.00
  0.2000000  0.1154701  0.0346980  12.00
  0.4000000  0.2309401  0.0346980  12.00
  0.2000000  0.3464102  0.0346980  12.00
  0.4000000  0.4618802  0.0346980  12.00
  0.0000000  0.0000000  0.0693960   2.00
  0.2000000  0.1154701  0.0693960  12.00
  0.4000000  0.2309401  0.0693960  12.00
  0.2000000  0.3464102  0.0693960  12.00
  0.4000000  0.4618802  0.0693960  12.00
TESR
  2 2 2
&END

&ATOMS
*Ti_MT_LDA_NLCC.psp KLEINMAN-BYLANDER NLCC
  LMAX=F  LOC=P
   6
          0.0000  0.00000 0.0000
          0.0000  0.33333 0.6666
          0.6666  0.33333 0.68520
          0.6666  0.33333 0.81480
          0.0000  0.0000  0.5000
          0.3333  0.6666  0.18520
*Si_MT_LDA.psp KLEINMAN-BYLANDER
 LMAX=D  LOC=P
  2
          0.000     0.00000      0.2500
          0.000     0.00000      0.7500
*C_GIA_LDA.psp KLEINMAN-BYLANDER
 LMAX=P   LOC=P
  4
          0.3333   0.6666  0.5723
          0.6666   0.3333  0.4277
          0.6666   0.3333  0.0723
          0.3333   0.6666  0.9277
&END

 PROGRAM CPMD STARTED AT: Thu Sep 23 09:17:20 2004



               ******  ******    ****  ****  ******
              *******  *******   **********  *******
             ***       **   ***  ** **** **  **   ***
             **        **   ***  **  **  **  **    **
             **        *******   **      **  **    **
             ***       ******    **      **  **   ***
              *******  **        **      **  *******
               ******  **        **      **  ******

                          VERSION 3.9.1

                            COPYRIGHT
                      IBM RESEARCH DIVISION
                MPI FESTKOERPERFORSCHUNG STUTTGART

                       The CPMD consortium
                    WWW:   http://www.cpmd.org
                 Mailinglist:   cpmd-list at cpmd.org
                     E-mail:   cpmd at cpmd.org


                  ***  Aug 13 2004 -- 13:52:08  ***

 THE INPUT FILE IS:                               Ti3SiC2.in.exec
 THIS JOB RUNS ON:
 THE CURRENT DIRECTORY IS:
                                      /home/eariel/mycpmd/Ti3SiC2
 THE TEMPORARY DIRECTORY IS:
                                      /home/eariel/mycpmd/Ti3SiC2
 THE PROCESS ID IS:                                          2700
 THE JOB WAS SUBMITTED BY:                                 eariel


 SINGLE POINT DENSITY OPTIMIZATION

 PATH TO THE RESTART FILES:                                    ./
 GRAM-SCHMIDT ORTHOGONALIZATION
 MAXIMUM NUMBER OF STEPS:                              1000 STEPS
 PRINT INTERMEDIATE RESULTS EVERY                     10001 STEPS
 STORE INTERMEDIATE RESULTS EVERY                     10001 STEPS
 NUMBER OF DISTINCT RESTART FILES:                              1
 TEMPERATURE IS CALCULATED ASSUMING EXTENDED BULK BEHAVIOR
 FICTITIOUS ELECTRON MASS:                               400.0000
 TIME STEP FOR ELECTRONS:                                  5.0000
 TIME STEP FOR IONS:                                       5.0000
 CONVERGENCE CRITERIA FOR WAVEFUNCTION OPTIMIZATION:   1.0000E-05
 WAVEFUNCTION OPTIMIZATION BY PRECONDITIONED DIIS
 THRESHOLD FOR THE WF-HESSIAN IS                           0.5000
 MAXIMUM NUMBER OF VECTORS RETAINED FOR DIIS:                  10
 STEPS UNTIL DIIS RESET ON POOR PROGRESS:                      10
 FULL ELECTRONIC GRADIENT IS USED
 SPLINE INTERPOLATION IN G-SPACE FOR PSEUDOPOTENTIAL FUNCTIONS
    NUMBER OF SPLINE POINTS:                                 5000

 EXCHANGE CORRELATION FUNCTIONALS
    LDA EXCHANGE:                                            NONE
    LDA XC THROUGH PADE APPROXIMATION
    S.GOEDECKER, J.HUTTER, M.TETER PRB 54 1703 (1996)

 ***     DETSP| THE NEW SIZE OF THE PROGRAM IS    2116/  24264 kBYTES ***

 ***************************** ATOMS ****************************
   NR   TYPE        X(bohr)        Y(bohr)        Z(bohr)     MBL
    1     Ti       0.000000       0.000000       0.000000       3
    2     Ti      -0.962963       1.667901      22.200167       3
    3     Ti       2.888543       1.667901      22.819614       3
    4     Ti       2.888543       1.667901      27.135758       3
    5     Ti       0.000000       0.000000      16.651790       3
    6     Ti       0.000000       3.335502       6.167823       3
    7     Si       0.000000       0.000000       8.325895       3
    8     Si       0.000000       0.000000      24.977686       3
    9      C       0.000000       3.335502      19.059639       3
   10      C       2.888630       1.667751      14.243942       3
   11      C       2.888630       1.667751       2.407849       3
   12      C       0.000000       3.335502      30.895732       3
 ****************************************************************

 NUMBER OF STATES:                                             24
 NUMBER OF ELECTRONS:                                    48.00000
 CHARGE:                                                  0.00000
 ELECTRON TEMPERATURE(KELVIN):                            0.00000
 OCCUPATION
  2.0  2.0  2.0  2.0  2.0  2.0  2.0  2.0  2.0  2.0  2.0  2.0  2.0
  2.0  2.0  2.0  2.0  2.0  2.0  2.0  2.0  2.0  2.0  2.0

    ============================================================
    |    Pseudopotential Report     Fri May 24 16:23:12 1996   |
    ------------------------------------------------------------
    |  Atomic Symbol                   :   TI                  |
    |  Atomic Number                   :  22                   |
    |  Number of core states           :   5                   |
    |  Number of valence states        :   2                   |
    |  Exchange-Correlation Functional :                       |
    |     Slater exchange :   .6667                            |
    |     LDA correlation : Ceperley-Alder                     |
    |  Electron Configuration :   N   L  Occupation            |
    |                             1   S    2.0000              |
    |                             2   S    2.0000              |
    |                             2   P    6.0000              |
    |                             3   S    2.0000              |
    |                             3   P    6.0000              |
    |                             3   D    2.0000              |
    |                             4   S    2.0000              |
    |  Full Potential Total Energy  -851.722440                |
    |  Trouiller-Martins normconserving PP                     |
    |     n    l        rc       energy                        |
    |     4    S    2.1000      -.16905                        |
    |     3    P    2.4000      -.16401                        |
    |     3    D    1.5000      -.16401                        |
    |     4    F    1.7076      -.16401                        |
    |  Nonlinear core correction                               |
    |  Core charge cutoff radius :   1.60000                   |
    |  Number of Mesh Points :   690                           |
    |  Pseudoatom Total Energy   -3.483142                     |
    ============================================================

    ============================================================
    |    Pseudopotential Report     Fri Dec  1 09:27:49 1995   |
    ------------------------------------------------------------
    |  Atomic Symbol                   :   SI                  |
    |  Atomic Number                   :  14                   |
    |  Number of core states           :   3                   |
    |  Number of valence states        :   2                   |
    |  Exchange-Correlation Functional :                       |
    |     Slater exchange :   .6667                            |
    |     LDA correlation : Ceperley-Alder                     |
    |  Electron Configuration :   N   L  Occupation            |
    |                             1   S    2.0000              |
    |                             2   S    2.0000              |
    |                             2   P    6.0000              |
    |                             3   S    2.0000              |
    |                             3   P    2.0000              |
    |  Full Potential Total Energy  -288.192200                |
    |  Trouiller-Martins normconserving PP                     |
    |     n    l        rc       energy                        |
    |     3    S    1.9000      -.39831                        |
    |     3    P    2.1000      -.15353                        |
    |     3    D    2.1000      -.15353                        |
    |  Number of Mesh Points :   664                           |
    |  Pseudoatom Total Energy   -3.745869                     |
    ============================================================

    ************************************************************
    *    CARBON LDA PSEUDOPOTENTIAL (CAR-VON BARTH TYPE)       *
    ************************************************************

 ****************************************************************
 *   ATOM       MASS   RAGGIO NLCC              PSEUDOPOTENTIAL *
 *     Ti    47.9000   1.2000  YES    KLEINMAN      S  NONLOCAL *
 *                                                  P     LOCAL *
 *                                                  D  NONLOCAL *
 *                                                  F  NONLOCAL *
 *     Si    28.0860   1.2000   NO    KLEINMAN      S  NONLOCAL *
 *                                                  P     LOCAL *
 *                                                  D  NONLOCAL *
 *      C    12.0112   1.2000   NO    KLEINMAN      S  NONLOCAL *
 *                                                  P     LOCAL *
 ****************************************************************


 OPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPEN
 NUMBER OF CPUS PER TASK                                        1
 OPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPEN

 ***     RGGEN| THE NEW SIZE OF THE PROGRAM IS    6732/  26988 kBYTES ***
 ***     RKPNT| THE NEW SIZE OF THE PROGRAM IS   18696/  38932 kBYTES ***

 ************************** SUPERCELL ***************************
 SYMMETRY:                                              HEXAGONAL
 LATTICE CONSTANT(a.u.):                                  5.77784
 CELL DIMENSION:   5.7778  1.0000  5.7640  0.0000  0.0000 -0.5000
 VOLUME(OMEGA IN BOHR^3):                               962.83566
 LATTICE VECTOR A1(BOHR):            5.7778     0.0000     0.0000
 LATTICE VECTOR A2(BOHR):           -2.8889     5.0038     0.0000
 LATTICE VECTOR A3(BOHR):            0.0000     0.0000    33.3036
 RECIP. LAT. VEC. B1(2Pi/BOHR):      0.1731     0.0999     0.0000
 RECIP. LAT. VEC. B2(2Pi/BOHR):      0.0000     0.1998     0.0000
 RECIP. LAT. VEC. B3(2Pi/BOHR):      0.0000     0.0000     0.0300
 REAL SPACE MESH:                    36           36          192
 WAVEFUNCTION CUTOFF(RYDBERG):                           80.00000
 DENSITY CUTOFF(RYDBERG):          (DUAL= 4.00)         320.00000
 NUMBER OF PLANE WAVES PER WAVEFUNCTION                     16433
 NUMBER OF PLANE WAVES AT GAMMA POINT                       11621
 NUMBER OF PLANE WAVES FOR DENSITY CUTOFF:                  46655
 KPOINTS (IN CARTESIAN COORDINATES AS INPUT):                  15
  NKP       KX           KY           KZ         WEIGHT       NGW
    1      0.00000      0.00000      0.00000    0.00800     11621
    2      0.20000      0.24880      0.00000    0.04800     11630
    3      0.40000      0.49761      0.00000    0.04800     11654
    4      0.20000      0.51547      0.00000    0.04800     11638
    5      0.40000      0.76427      0.00000    0.04800     11636
    6      0.00000      0.00000      0.00602    0.01600     11615
    7      0.20000      0.24880      0.00602    0.09600     11632
    8      0.40000      0.49761      0.00602    0.09600     11656
    9      0.20000      0.51547      0.00602    0.09600     11631
   10      0.40000      0.76427      0.00602    0.09600     11636
   11      0.00000      0.00000      0.01204    0.01600     11621
   12      0.20000      0.24880      0.01204    0.09600     11632
   13      0.40000      0.49761      0.01204    0.09600     11652
   14      0.20000      0.51547      0.01204    0.09600     11630
   15      0.40000      0.76427      0.01204    0.09600     11636
 [K-POINTS IN INPUT FILE WERE IN RECIPROCAL COORDINATES]
 ****************************************************************

 ***  RINFORCE| THE NEW SIZE OF THE PROGRAM IS  113624/ 134600 kBYTES ***
 ***    FFTPRP| THE NEW SIZE OF THE PROGRAM IS  107652/ 126328 kBYTES ***

 GENERATE ATOMIC BASIS SET
     Ti        SLATER ORBITALS
        3D        ALPHA=   3.8833      OCCUPATION= 2.00
        4S        ALPHA=   0.8514      OCCUPATION= 2.00
     Si        SLATER ORBITALS
        3S        ALPHA=   1.6344      OCCUPATION= 2.00
        3P        ALPHA=   1.4284      OCCUPATION= 2.00
      C        SLATER ORBITALS
        2S        ALPHA=   1.6083      OCCUPATION= 2.00
        2P        ALPHA=   1.5679      OCCUPATION= 2.00


 INITIALIZATION TIME:                                7.02 SECONDS

 ***    WFOPTS| THE NEW SIZE OF THE PROGRAM IS  109044/ 816036 kBYTES ***
 ***     PHFAC| THE NEW SIZE OF THE PROGRAM IS  109236/ 885192 kBYTES ***
 ***    ATOMWF| THE NEW SIZE OF THE PROGRAM IS  157020/ 902264 kBYTES ***
  ATRHO| CHARGE(R-SPACE):   48.000000      (G-SPACE):   48.000000

 ****************************************************************
 *                      ATOMIC COORDINATES                      *
 ****************************************************************
       1      Ti           0.000000       0.000000       0.000000
       2      Ti          -0.962963       1.667901      22.200167
       3      Ti           2.888543       1.667901      22.819614
       4      Ti           2.888543       1.667901      27.135758
       5      Ti           0.000000       0.000000      16.651790
       6      Ti           0.000000       3.335502       6.167823
       7      Si           0.000000       0.000000       8.325895
       8      Si           0.000000       0.000000      24.977686
       9       C           0.000000       3.335502      19.059639
      10       C           2.888630       1.667751      14.243942
      11       C           2.888630       1.667751       2.407849
      12       C           0.000000       3.335502      30.895732
 ****************************************************************


 DEGREES OF FREEDOM FOR SYSTEM:                                33

 CPU TIME FOR WAVEFUNCTION INITIALIZATION:         184.08 SECONDS
 ***    RWFOPT| THE NEW SIZE OF THE PROGRAM IS  266440/ 888700 kBYTES ***
  EWALD| SUM IN REAL SPACE OVER                     5* 5* 5 CELLS

 TOTAL INTEGRATED ELECTRONIC DENSITY
    IN G-SPACE =                                        48.000000
    IN R-SPACE =                                        48.000000

 (K+E1+L+N+X)           TOTAL ENERGY =        -1192.80202568 A.U.
 (K)                  KINETIC ENERGY =           67.27338193 A.U.
 (E1=A-S+R)     ELECTROSTATIC ENERGY =          -36.67936117 A.U.
 (S)                           ESELF =           63.83076486 A.U.
 (R)                             ESR =            0.82722476 A.U.
 (L)    LOCAL PSEUDOPOTENTIAL ENERGY =          -15.98904416 A.U.
 (N)      N-L PSEUDOPOTENTIAL ENERGY =        -1188.59318419 A.U.
 (X)     EXCHANGE-CORRELATION ENERGY =          -23.25101640 A.U.

 NFI      GEMAX       CNORM           ETOT        DETOT      TCPU
   1  1.397E+02   3.172E+00   -1192.802026    0.000E+00     81.95
   2  2.564E+02   5.572E+00  -16804.228069   -1.561E+04     83.28
   3  4.043E+02   6.379E+00  -13463.052701    3.341E+03     84.43
   4  3.094E+02   5.203E+00  -18043.217053   -4.580E+03     85.65
   5  3.440E+02   5.897E+00  -17045.966609    9.973E+02     86.92
   6  2.963E+02   5.573E+00  -16785.896226    2.601E+02     88.20
   7  2.743E+02   5.710E+00  -16797.347620   -1.145E+01     89.49
   8  2.205E+02   4.944E+00  -18592.872219   -1.796E+03     90.82
   9  2.896E+02   5.080E+00  -17588.452522    1.004E+03     92.17
  10  2.545E+02   4.874E+00  -18229.351795   -6.409E+02     93.37
  11  2.674E+02   5.032E+00  -18012.594573    2.168E+02     93.40
 ODIIS| Insufficient progress; reset!


Eduardo A. Menendez Proupin
Department of Physics
Faculty of Science
University of Chile
Las Palmeras 3425
Ñuñoa, Santiago
Chile
Phone: 56+2+678 74 11
http://fisica.ciencias.uchile.cl/~emenendez/




More information about the CPMD-list mailing list