[CPMD-list] free isolated atom energiesB

Ari P Seitsonen Ari.P.Seitsonen at iki.fi
Fri Sep 17 02:04:33 CEST 2004


Dear Eduardo,

  Just some thoughts:

 1) Like you noticed, the occupation numbers 2, 2, 1, 1 do not make really
   sense; well, this is leads to a non-spherical atom (p_x, p_y and p_z
   are occupied differently), which is used in the pseudo potential
   program. You should use an equal occupation of the p levels if you want
   to compare with Paolo Giannozzi's program (hmm, keyword 'OCCUPATION'?)

 2) Vanderbilt: The calculation is not fully converged, and the occupation
    numbers are 2, 2, 2. I'd first try with the pre-given occupation
    numbers. Still I'm a bit worried why some of the p levels have a
    positive eigenvalue, maybe the zero is not at the vacuum level (like
    in the case of an isolated molecule with a norm-conserving potential;
    something wrong in the diagonalisation with Vdb pp's?)

  Hopefully this helps something.

    Greetings,

       apsi

-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-
 Ari Paavo Seitsonen / Ari.P.Seitsonen at iki.fi / http://www.iki.fi/~apsi/
 Tel +41 1 635 44 97 / Fax +41 1 635 68 38 / GSM +41 79 719 09 35      
 Anschrift: Physikalisch Chemisches Institut (PCI), Universität Zürich (UniZh)
 Indirizzo: Winterthurerstrasse 190, CH-8057 Zürich
 Address:   Schweiz / Svizzera / Suisse / Svizra / Switzerland

On Thu, 16 Sep 2004, Eduardo Ariel Menendez P wrote:

> Hello everybody:
> 
> During last days I have been involved in generation and testing of
> pseudopotentials for Cd and Te.  After having performed the tests
> available in the pseudopp generation package (Giannozzi's) and convert the
> pseudopotentials to CPMD format, I find that the energies of the isolated
> atoms do not coincide precisely. The greatest difference betwwen CPMD and
> the atomic
> package is for the Te 5p level, where I found a difference of nearly
> 0.7eV, while 0.01 difference for Te 5s.  I have tried increasing the
> cutoff and the lattice constant without improvement.
> Hence, I decided to
> use a database pseupotencial with the most common element on Earth: O.
> 
> Even so I have two problems
> 
> 1) Using a supplied MT pseudopotential (O_MT_LDA.psp)
> I have found .
> EIGENVALUES(EV) AND OCCUPATION:
>  1    -23.9467297NC   2.000        2     -8.7260317NC   2.000
>  3     -8.7260316NC   2.000
>  CHEMICAL POTENTIAL =                            -8.7260316211 EV
> 
> The energies are not precise, compared wih available references:
> 
> http://physics.nist.gov/PhysRefData/DFTdata/Tables/08O.html
> 2s     -0.871362 Ha= -23.70104 eV
> 2p     -0.338381 Ha = -9.20 eV
> 
> And the output of the atomic pp  generation package og Giannozzi
> n l     nl            e(Ry)      (eV)
> 1 0     1S( 2.00)   -37.5178   -510.4594
> 2 0     2S( 2.00)    -1.7424    -23.7069
> 2 1     2P( 4.00)    -0.6766     -9.2055
> 
> E(2P)-E(2S)=14.50eV
> 
> CPMD: E(2P)-E(2S)=15.22eV.
> 
> 
> Morevoer, if I calculate Kohn-Sham empty state energies I find
> 
>  EIGENVALUES(EV) AND OCCUPATION:
>  1    -23.9412023     2.000        2    -10.3153247     2.000
>  3     -8.7206696     1.000        4     -8.7206695     1.000
>  5     -0.5820744     0.000
> CHEMICAL POTENTIAL =                            -8.7206708302 EV
> 
> I would expect that the energies of the states 2,3 and 4 be equal, corresponding to the
> three 2p levels. However, the state 2 has a differente.  It is interesting that the
> occupation factors of 3 and 4 are 1, even when I am using LDA and not LSD. I guess  it may be
> associated to the quasi-degeneracy.
> Here is the input file of the last calculation
> 
> &CPMD
>   RESTART DENSITY
>   KOHN-SHAM ENERGIES
>    2
>   MAXSTEP
>   150
>   CENTER MOLECULE ON
> &END
> 
> &DFT
>   NEWCODE
>   FUNCTIONAL LDA
>   LDA CORRELATION PZ
>   SLATER
>     0.666667
>   GC-CUTOFF
>   0.1E-07
> &END
> 
> &SYSTEM
>   SYMMETRY
>   0
>   ANGSTROM
>   CELL
>     8.0  1.0  1.0  0  0  0
>   CUTOFF SPHERICAL
>     95.0
> &END
> 
> &ATOMS
> *O_MT_LDA.psp KLEINMAN-BYLANDER
>    LMAX=D LOC=D     #Also tried with LOC=P and LOC=S
>    1
>     0.000000    0.000000    0.000000
> &END
> 
> 
> 
> 
> 2) SECOND PROBLEM
> The second test I did was using ultrasoft pp.
> For example,
> performing optimization of the wavefunction  for one O in a box of 8 Angstroms, and then calculating the Khon-Sham energies I found striking diferences:
> 
> With this entry
> &CPMD
>   RESTART DENSITY
>   KOHN-SHAM ENERGIES
>      0
> output:
>  EIGENVALUES(EV) AND OCCUPATION:
>  1    -11.2781946     2.000        2      0.7058206     2.000
>  3      0.7065389NC   2.000
>  CHEMICAL POTENTIAL =                             0.7065371502 EV
> *********************************
> With the same RESTART file and this  input
> &CPMD
>  RESTART DENSITY
>  KOHN-SHAM ENERGIES
>    2
> y get this outpput:
> EIGENVALUES(EV) AND OCCUPATION:
>  1    -11.2781946     2.000        2     -0.3815193     2.000
>  3     -0.2300328     2.000        4      0.7065208     0.000
>  5      0.7065390     0.000
>  CHEMICAL POTENTIAL =                            -0.2300326449 EV
> 
> First problem: The energies do not seem to be correct. Now the "P energy is terribly wrong
> 
> http://physics.nist.gov/PhysRefData/DFTdata/Tables/08O.html
> 2s     -0.871362 Ha= -23.70104 eV
> 2p     -0.338381 Ha = -9.20 eV
> 
> Also, the states 2,3,and 4 have all diferent energies.
> 
> 
> Follow full input and output  files with the USPP.
> 
> 1) Optimization
> &CPMD
>   INITIALIZE WAVEFUNCTION RANDOM
>   OPTIMIZE WAVEFUNCTION
>   MAXSTEP
>   150
>   CENTER MOLECULE ON
> &END
> 
> 
> &DFT
>   NEWCODE
>   FUNCTIONAL LDA
>   LDA CORRELATION PZ
>   SLATER
>     0.666667
>   GC-CUTOFF
>   0.1E-07
> &END
> 
> &SYSTEM
>   SYMMETRY
>   0
>   ANGSTROM
>   CELL
>     8.0  1.0  1.0  0  0  0
>   CUTOFF SPHERICAL
>     55.0
> &END
> 
> &ATOMS
> *O_VDB_LDA.psp FORMATTED
>    LMAX=P LOC=P
>    1
>     0.000000    0.000000    0.000000
> &END
> 
> 2) KS orbitals. Only occ states
> 
> &CPMD
>   RESTART DENSITY
>   KOHN-SHAM ENERGIES
>    0
>   MAXSTEP
>   150
>   CENTER MOLECULE ON
> &END
> 
> 
> &DFT
>   NEWCODE
>   FUNCTIONAL LDA
>   LDA CORRELATION PZ
>   SLATER
>     0.666667
>   GC-CUTOFF
>   0.1E-07
> &END
> 
> &SYSTEM
>   SYMMETRY
>   0
>   ANGSTROM
>   CELL
>     8.0  1.0  1.0  0  0  0
>   CUTOFF SPHERICAL
>     55.0
> &END
> 
> &ATOMS
> *O_VDB_LDA.psp FORMATTED
>    LMAX=D LOC=D
>    1
>     0.000000    0.000000    0.000000
> &END
>  PROGRAM CPMD STARTED AT: Fri Sep 17 00:46:21 2004
> 
> 
> 
>                ******  ******    ****  ****  ******
>               *******  *******   **********  *******
>              ***       **   ***  ** **** **  **   ***
>              **        **   ***  **  **  **  **    **
>              **        *******   **      **  **    **
>              ***       ******    **      **  **   ***
>               *******  **        **      **  *******
>                ******  **        **      **  ******
> 
>                           VERSION 3.9.1
> 
>                             COPYRIGHT
>                       IBM RESEARCH DIVISION
>                 MPI FESTKOERPERFORSCHUNG STUTTGART
> 
>                        The CPMD consortium
>                     WWW:   http://www.cpmd.org
>                  Mailinglist:   cpmd-list at cpmd.org
>                      E-mail:   cpmd at cpmd.org
> 
> 
>                   ***  Aug 13 2004 -- 13:52:08  ***
> 
>  THE INPUT FILE IS:                                         o.inp
>  THIS JOB RUNS ON:
>  THE CURRENT DIRECTORY IS:
>                                             /home/eariel/mycpmd/O
>  THE TEMPORARY DIRECTORY IS:
>                                             /home/eariel/mycpmd/O
>  THE PROCESS ID IS:                                          2530
>  THE JOB WAS SUBMITTED BY:                                 eariel
> 
> 
>  SINGLE POINT DENSITY OPTIMIZATION
> 
> 
>  EXACT DIAGONALIZATION OF KOHN-SHAM MATRIX
> 
>  PATH TO THE RESTART FILES:                                    ./
>  RESTART WITH OLD DENSITY
>  GRAM-SCHMIDT ORTHOGONALIZATION
>  MAXIMUM NUMBER OF STEPS:                                 1 STEPS
>  MAXIMUM NUMBER OF ITERATIONS FOR SC:                     1 STEPS
>  PRINT INTERMEDIATE RESULTS EVERY                     10001 STEPS
>  STORE INTERMEDIATE RESULTS EVERY                     10001 STEPS
>  STORE ELECTRONIC DENSITY IN RESTART FILE
>  NUMBER OF DISTINCT RESTART FILES:                              1
>  TEMPERATURE IS CALCULATED ASSUMING EXTENDED BULK BEHAVIOR
>  TIME STEP FOR ELECTRONS:                                  5.0000
>  TIME STEP FOR IONS:                                       5.0000
>  CONVERGENCE CRITERIA FOR WAVEFUNCTION OPTIMIZATION:   1.0000E-03
>  LANCZOS DIAGONALIZATION (KRYLOV SUBSPACE)
>     MAX. FRIESNER ITERATIONS                                  200
>     MAX. KRYLOV SUBSPACE                                        6
>     MAX. KRYLOV BLOCK SIZE       FIXED LATER (WAITING FOR NSTATE)
>     MAX. BETA^2                                        1.0000E-08
>  ANDERSON MIXING PARAMETER:                            2.0000E-01
>  BROYDEN MIXING PARAMETER [BROYMIX]                    1.5000E-01
>  BROYDEN CUTOFF [ECUTBROY]            EQUAL TO THE DENSITY CUTOFF
>  BROYDEN MIXING STARTS [NFRBROY] AFTER                    0 STEPS
>  BROYDEN MIXING RESET [IBRESET] AFTER                     8 STEPS
>  BROYDEN MIXING W02                                    1.0000E-02
>  ALEXANDER MIXING:                                         0.9000
>  SPLINE INTERPOLATION IN G-SPACE FOR PSEUDOPOTENTIAL FUNCTIONS
>     NUMBER OF SPLINE POINTS:                                 5000
> 
>  EXCHANGE CORRELATION FUNCTIONALS
>     LDA EXCHANGE:                        SLATER (ALPHA = 0.66667)
>     LDA CORRELATION:                              PERDEW & ZUNGER
>        [J.P. PERDEW AND A ZUNGER, PRB 23 5048 (1981)]
> 
>  ***     DETSP| THE NEW SIZE OF THE PROGRAM IS    1940/  22060 kBYTES ***
> 
>  >>>>>>>> CENTER OF MASS HAS BEEN MOVED TO CENTER OF BOX <<<<<<<<
> 
> 
>  ***************************** ATOMS ****************************
>    NR   TYPE        X(bohr)        Y(bohr)        Z(bohr)     MBL
>     1      O       7.558904       7.558904       7.558904       3
>  ****************************************************************
> 
>  NUMBER OF STATES:                                              3
>  NUMBER OF ELECTRONS:                                     6.00000
>  CHARGE:                                                  0.00000
>  ELECTRON TEMPERATURE(KELVIN):                            0.00000
>  OCCUPATION
>   2.0  2.0  2.0
> 
>  LANCZOS DIAGONALIZATION (KRYLOV SUBSPACE)
>     MAX. KRYLOV BLOCK SIZE                                      3
> 
>    ============================================================
>    |  pseudopotential report: version  7.3.4 date  6-12-2003  |
>    ------------------------------------------------------------
>    |  oxygen                    ceperley-alder exchange-corr  |
>    |  z =   8.00  zv =   6.00  exfact =   0.00000             |
>    |                            etot  = -31.51046             |
>    |  index    orbital      occupation    energy              |
>    |    1        200           2.00       -1.74               |
>    |    2        210           4.00       -0.68               |
>    |  keyps = 3     ifpcor = 0                                |
>    |  rinner =      0.80     for L=    1                      |
>    |  rinner =      0.80     for L=    2                      |
>    |  rinner =      0.80     for L=    3                      |
>    |    new generation scheme:                                |
>    |    nbeta =  4     kkbeta =  507     rcloc =    1.0000    |
>    |    ibeta     l     epsilon   rcut iptype                 |
>    |       1      0      -1.74   1.10      2                  |
>    |       2      0      -0.20   1.10      2                  |
>    |       3      1      -0.80   1.10      2                  |
>    |       4      1       0.20   1.10      2                  |
>    |  npf    = 8  ptryc =  10.000                             |
>    |  lloc   = 2  eloc   =   0.000                            |
>    |  ifqopt = 2  nqf    = 8  qtryc =  10.000                 |
>    |  all electron calculation used schroedinger equation     |
>    |         ************logarithmic mesh************         |
>    ============================================================
> 
>  ****************************************************************
>  *   ATOM       MASS   RAGGIO NLCC              PSEUDOPOTENTIAL *
>  *     O     15.9994   1.2000   NO              VANDERBILT      *
>  ****************************************************************
> 
> 
>  OPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPEN
>  NUMBER OF CPUS PER TASK                                        1
>  OPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPEN
> 
>  ***     RGGEN| THE NEW SIZE OF THE PROGRAM IS    8656/  36592 kBYTES ***
> 
>  ************************** SUPERCELL ***************************
>  THIS IS AN ISOLATED SYSTEM CALCULATION
>  POISSON EQUATION SOLVER  :                               HOCKNEY
>  COULOMB SMOOTHING RADIUS :                                 1.080
>  SYMMETRY:                                           SIMPLE CUBIC
>  LATTICE CONSTANT(a.u.):                                 15.11781
>  CELL DIMENSION:  15.1178  1.0000  1.0000  0.0000  0.0000  0.0000
>  VOLUME(OMEGA IN BOHR^3):                              3455.14651
>  LATTICE VECTOR A1(BOHR):           15.1178     0.0000     0.0000
>  LATTICE VECTOR A2(BOHR):            0.0000    15.1178     0.0000
>  LATTICE VECTOR A3(BOHR):            0.0000     0.0000    15.1178
>  RECIP. LAT. VEC. B1(2Pi/BOHR):      0.0661     0.0000     0.0000
>  RECIP. LAT. VEC. B2(2Pi/BOHR):      0.0000     0.0661     0.0000
>  RECIP. LAT. VEC. B3(2Pi/BOHR):      0.0000     0.0000     0.0661
>  REAL SPACE MESH:                    72           72           72
>  WAVEFUNCTION CUTOFF(RYDBERG):                           55.00000
>  DENSITY CUTOFF(RYDBERG):          (DUAL= 4.00)         220.00000
>  NUMBER OF PLANE WAVES FOR WAVEFUNCTION CUTOFF:             11924
>  NUMBER OF PLANE WAVES FOR DENSITY CUTOFF:                  95160
>  NUMBER OF PLANE WAVES FOR BROYDEN MIXING:                  95160
>  ****************************************************************
> 
>  ***  RINFORCE| THE NEW SIZE OF THE PROGRAM IS   19336/  48876 kBYTES ***
>  ***    FFTPRP| THE NEW SIZE OF THE PROGRAM IS   30400/  50196 kBYTES ***
>  ***   CLUSTER| THE NEW SIZE OF THE PROGRAM IS   34304/  53980 kBYTES ***
> 
>  GENERATE ATOMIC BASIS SET
>       O        SLATER ORBITALS
>         2S        ALPHA=   2.2458      OCCUPATION= 2.00
>         2P        ALPHA=   2.2266      OCCUPATION= 4.00
> 
> 
>  INITIALIZATION TIME:                               13.06 SECONDS
> 
>  ***    WFOPTS| THE NEW SIZE OF THE PROGRAM IS   34520/  60124 kBYTES ***
>  RV30| WARNING! NO DENSITY INFORMATION
> 
>  RESTART INFORMATION READ ON FILE                       ./RESTART
>  ***     PHFAC| THE NEW SIZE OF THE PROGRAM IS   34780/  89428 kBYTES ***
>  ***    ATOMWF| THE NEW SIZE OF THE PROGRAM IS   34984/  90924 kBYTES ***
>   ATRHO| CHARGE(R-SPACE):    6.000000      (G-SPACE):    6.000000
> 
>  ****************************************************************
>  *                      ATOMIC COORDINATES                      *
>  ****************************************************************
>        1       O           7.558904       7.558904       7.558904
>  ****************************************************************
> 
>   !! WARNING FROM DETDOF: WHY IS GLIB LESS THAN UNITY !!
>   !! WARNING FROM DETDOF: NOW IT IS SET EQUAL TO UNITY !!
> 
>  DEGREES OF FREEDOM FOR SYSTEM:                                 1
> 
>  CPU TIME FOR WAVEFUNCTION INITIALIZATION:           3.44 SECONDS
>  ***    RWFOPT| THE NEW SIZE OF THE PROGRAM IS   64920/  89564 kBYTES ***
>   EWALD| SUM IN REAL SPACE OVER                     1* 1* 1 CELLS
> 
>  <<<<<<<<<<<<<<<<<<< LANCZOS DIAGONALIZATION <<<<<<<<<<<<<<<<<<<<
>  >> TIME FOR INITIAL SUBSPACE DIAGONALIZATION:               0.32
>  >> CYCLE     NCONV        B2MAX        B2MIN     #HPSI      TIME
>         1         0    1.561E-01    4.184E-02      6.00      1.58
>         2         0    1.562E-01    8.824E-03      5.00      1.57
>         3         0    6.681E-02    2.637E-03      5.00      1.58
>         4         0    5.009E-02    8.258E-04      5.00      1.57
>         5         0    2.734E-02    2.903E-04      5.00      1.58
>         6         0    2.382E-02    1.033E-04      5.00      1.57
>         7         0    1.440E-02    3.971E-05      5.00      1.58
>         8         0    1.340E-02    1.528E-05      5.00      1.57
>         9         0    8.514E-03    4.825E-06      5.00      1.58
>        10         0    8.230E-03    2.850E-06      5.00      1.57
>        11         0    5.415E-03    1.034E-06      5.00      1.57
>        12         0    5.390E-03    6.196E-07      5.00      1.57
>        13         0    3.644E-03    2.334E-07      5.00      1.58
>        14         0    3.711E-03    1.416E-07      5.00      1.57
>        15         0    2.561E-03    5.407E-08      5.00      1.57
>        16         0    2.654E-03    3.308E-08      5.00      1.58
>        17         0    1.859E-03    1.274E-08      5.00      1.57
>        18         1    1.950E-03    9.159E-09      4.00      1.13
>        19         1    1.380E-03    9.159E-09      3.33      0.82
>        20         1    1.459E-03    9.159E-09      3.33      0.83
>        21         1    1.039E-03    9.159E-09      3.33      0.83
>        22         1    1.104E-03    9.159E-09      3.33      0.82
>        23         1    7.904E-04    9.159E-09      3.33      0.83
>        24         1    8.425E-04    9.159E-09      3.33      0.82
>        25         1    6.047E-04    9.159E-09      3.33      0.83
>        26         1    6.459E-04    9.159E-09      3.33      0.83
>        27         1    4.644E-04    9.159E-09      3.33      0.82
>        28         1    4.966E-04    9.159E-09      3.33      0.83
>        29         1    3.574E-04    9.159E-09      3.33      0.83
>        30         1    3.824E-04    9.159E-09      3.33      0.82
>        31         1    2.754E-04    9.159E-09      3.33      0.83
>        32         1    2.948E-04    9.159E-09      3.33      0.83
>        33         1    2.124E-04    9.159E-09      3.33      0.82
>        34         1    2.274E-04    9.159E-09      3.33      0.83
>        35         1    1.639E-04    9.159E-09      3.33      0.82
>        36         1    1.755E-04    9.159E-09      3.33      0.83
>        37         1    1.265E-04    9.159E-09      3.33      0.83
>        38         1    1.354E-04    9.159E-09      3.33      0.82
>        39         1    9.763E-05    9.159E-09      3.33      0.83
>        40         1    1.045E-04    9.159E-09      3.33      0.83
>        41         1    7.535E-05    9.159E-09      3.33      0.82
>        42         1    8.067E-05    9.159E-09      3.33      0.83
>        43         1    5.816E-05    9.159E-09      3.33      0.82
>        44         1    6.227E-05    9.159E-09      3.33      0.83
>        45         1    4.489E-05    9.159E-09      3.33      0.83
>        46         1    4.806E-05    9.159E-09      3.33      0.82
>        47         1    3.465E-05    9.159E-09      3.33      0.83
>        48         1    3.709E-05    9.159E-09      3.33      0.82
>        49         1    2.675E-05    9.159E-09      3.33      0.82
>        50         1    2.863E-05    9.159E-09      3.33      0.83
>        51         1    2.064E-05    9.159E-09      3.33      0.82
>        52         1    2.210E-05    9.159E-09      3.33      0.83
>        53         1    1.593E-05    9.159E-09      3.33      0.83
>        54         1    1.706E-05    9.159E-09      3.33      0.82
>        55         1    1.230E-05    9.159E-09      3.33      0.83
>        56         1    1.317E-05    9.159E-09      3.33      0.82
>        57         1    9.494E-06    9.159E-09      3.33      0.83
>        58         1    1.016E-05    9.159E-09      3.33      0.83
>        59         1    7.329E-06    9.159E-09      3.33      0.82
>        60         1    7.844E-06    9.159E-09      3.33      0.82
>        61         1    5.657E-06    9.159E-09      3.33      0.83
>        62         1    6.055E-06    9.159E-09      3.33      0.82
>        63         1    4.367E-06    9.159E-09      3.33      0.83
>        64         1    4.674E-06    9.159E-09      3.33      0.83
>        65         1    3.371E-06    9.159E-09      3.33      0.82
>        66         1    3.609E-06    9.159E-09      3.33      0.82
>        67         1    2.603E-06    9.159E-09      3.33      0.82
>        68         1    2.786E-06    9.159E-09      3.33      0.83
>        69         1    2.010E-06    9.159E-09      3.33      0.83
>        70         1    2.151E-06    9.159E-09      3.33      0.82
>        71         1    1.552E-06    9.159E-09      3.33      0.83
>        72         1    1.661E-06    9.159E-09      3.33      0.82
>        73         1    1.198E-06    9.159E-09      3.33      0.83
>        74         1    1.283E-06    9.159E-09      3.33      0.83
>        75         1    9.256E-07    9.159E-09      3.33      0.83
>        76         1    9.910E-07    9.159E-09      3.33      0.82
>        77         1    7.151E-07    9.159E-09      3.33      0.83
>        78         1    7.657E-07    9.159E-09      3.33      0.82
>        79         1    5.526E-07    9.159E-09      3.33      0.83
>        80         1    5.919E-07    9.159E-09      3.33      0.82
>        81         1    4.273E-07    9.159E-09      3.33      0.83
>        82         1    4.578E-07    9.159E-09      3.33      0.82
>        83         1    3.307E-07    9.159E-09      3.33      0.82
>        84         1    3.544E-07    9.159E-09      3.33      0.83
>        85         1    2.561E-07    9.159E-09      3.33      0.82
>        86         1    2.748E-07    9.159E-09      3.33      0.83
>        87         1    1.987E-07    9.159E-09      3.33      0.83
>        88         1    2.134E-07    9.159E-09      3.33      0.82
>        89         1    1.545E-07    9.159E-09      3.33      0.83
>        90         1    1.662E-07    9.159E-09      3.33      0.83
>        91         1    1.205E-07    9.159E-09      3.33      0.82
>        92         1    1.299E-07    9.159E-09      3.33      0.83
>        93         1    9.449E-08    9.159E-09      3.33      0.82
>        94         1    1.021E-07    9.159E-09      3.33      0.83
>        95         1    7.456E-08    9.159E-09      3.33      0.83
>        96         1    8.096E-08    9.159E-09      3.33      0.82
>        97         1    5.940E-08    9.159E-09      3.33      0.83
>        98         1    6.490E-08    9.159E-09      3.33      0.83
>        99         1    4.796E-08    9.159E-09      3.33      0.82
>       100         1    5.283E-08    9.159E-09      3.33      0.83
>       101         1    3.942E-08    9.159E-09      3.33      0.82
>       102         1    4.391E-08    9.159E-09      3.33      0.83
>       103         1    3.317E-08    9.159E-09      3.33      0.83
>       104         1    3.747E-08    9.159E-09      3.33      0.82
>       105         1    2.874E-08    9.159E-09      3.33      0.83
>       106         1    3.302E-08    9.159E-09      3.33      0.83
>       107         2    2.578E-08    9.159E-09      2.33      0.78
>       108         2    3.019E-08    9.159E-09      1.67      0.75
>       109         2    2.403E-08    9.159E-09      1.67      0.75
>       110         2    2.871E-08    9.159E-09      1.67      0.75
>       111         2    2.330E-08    9.159E-09      1.67      0.75
>       112         2    2.838E-08    9.159E-09      1.67      0.76
>       113         2    2.345E-08    9.159E-09      1.67      0.75
>       114         2    2.906E-08    9.159E-09      1.67      0.75
>       115         2    2.439E-08    9.159E-09      1.67      0.75
>       116         2    3.066E-08    9.159E-09      1.67      0.75
>       117         2    2.606E-08    9.159E-09      1.67      0.75
>       118         2    3.313E-08    9.159E-09      1.67      0.75
>       119         2    2.843E-08    9.159E-09      1.67      0.75
>       120         2    3.644E-08    9.159E-09      1.67      0.76
>       121         2    3.149E-08    9.159E-09      1.67      0.75
>       122         2    4.062E-08    9.159E-09      1.67      0.75
>       123         2    3.527E-08    9.159E-09      1.67      0.75
>       124         2    4.569E-08    9.159E-09      1.67      0.75
>       125         2    3.981E-08    9.159E-09      1.67      0.75
>       126         2    5.172E-08    9.159E-09      1.67      0.75
>       127         2    4.518E-08    9.159E-09      1.67      0.75
>       128         2    5.880E-08    9.159E-09      1.67      0.76
>       129         2    5.145E-08    9.159E-09      1.67      0.75
>       130         2    6.705E-08    9.159E-09      1.67      0.75
>       131         2    5.873E-08    9.159E-09      1.67      0.75
>       132         2    7.660E-08    9.159E-09      1.67      0.75
>       133         2    6.715E-08    9.159E-09      1.67      0.75
>       134         2    8.763E-08    9.159E-09      1.67      0.75
>       135         2    7.685E-08    9.159E-09      1.67      0.75
>       136         2    1.003E-07    9.159E-09      1.67      0.74
>       137         2    8.803E-08    9.159E-09      1.67      0.76
>       138         2    1.150E-07    9.159E-09      1.67      0.75
>       139         2    1.009E-07    9.159E-09      1.67      0.75
>       140         2    1.317E-07    9.159E-09      1.67      0.75
>       141         2    1.156E-07    9.159E-09      1.67      0.75
>       142         2    1.510E-07    9.159E-09      1.67      0.75
>       143         2    1.326E-07    9.159E-09      1.67      0.75
>       144         2    1.732E-07    9.159E-09      1.67      0.75
>       145         2    1.520E-07    9.159E-09      1.67      0.74
>       146         2    1.986E-07    9.159E-09      1.67      0.75
>       147         2    1.743E-07    9.159E-09      1.67      0.75
>       148         2    2.277E-07    9.159E-09      1.67      0.75
>       149         2    1.999E-07    9.159E-09      1.67      0.75
>       150         2    2.611E-07    9.159E-09      1.67      0.75
>       151         2    2.293E-07    9.159E-09      1.67      0.75
>       152         2    2.995E-07    9.159E-09      1.67      0.75
>       153         2    2.629E-07    9.159E-09      1.67      0.75
>       154         2    3.434E-07    9.159E-09      1.67      0.75
>       155         2    3.015E-07    9.159E-09      1.67      0.75
>       156         2    3.939E-07    9.159E-09      1.67      0.75
>       157         2    3.458E-07    9.159E-09      1.67      0.75
>       158         2    4.517E-07    9.159E-09      1.67      0.75
>       159         2    3.966E-07    9.159E-09      1.67      0.75
>       160         2    5.181E-07    9.159E-09      1.67      0.75
>       161         2    4.549E-07    9.159E-09      1.67      0.75
>       162         2    5.941E-07    9.159E-09      1.67      0.75
>       163         2    5.217E-07    9.159E-09      1.67      0.75
>       164         2    6.814E-07    9.159E-09      1.67      0.75
>       165         2    5.983E-07    9.159E-09      1.67      0.75
>       166         2    7.815E-07    9.159E-09      1.67      0.75
>       167         2    6.862E-07    9.159E-09      1.67      0.75
>       168         2    8.963E-07    9.159E-09      1.67      0.75
>       169         2    7.870E-07    9.159E-09      1.67      0.75
>       170         2    1.028E-06    9.159E-09      1.67      0.75
>       171         2    9.026E-07    9.159E-09      1.67      0.75
>       172         2    1.179E-06    9.159E-09      1.67      0.75
>       173         2    1.035E-06    9.159E-09      1.67      0.75
>       174         2    1.352E-06    9.159E-09      1.67      0.76
>       175         2    1.187E-06    9.159E-09      1.67      0.75
>       176         2    1.551E-06    9.159E-09      1.67      0.75
>       177         2    1.362E-06    9.159E-09      1.67      0.75
>       178         2    1.778E-06    9.159E-09      1.67      0.75
>       179         2    1.562E-06    9.159E-09      1.67      0.75
>       180         2    2.039E-06    9.159E-09      1.67      0.75
>       181         2    1.791E-06    9.159E-09      1.67      0.75
>       182         2    2.339E-06    9.159E-09      1.67      0.76
>       183         2    2.054E-06    9.159E-09      1.67      0.74
>       184         2    2.682E-06    9.159E-09      1.67      0.74
>       185         2    2.356E-06    9.159E-09      1.67      0.75
>       186         2    3.076E-06    9.159E-09      1.67      0.75
>       187         2    2.701E-06    9.159E-09      1.67      0.75
>       188         2    3.528E-06    9.159E-09      1.67      0.74
>       189         2    3.098E-06    9.159E-09      1.67      0.75
>       190         2    4.046E-06    9.159E-09      1.67      0.75
>       191         2    3.553E-06    9.159E-09      1.67      0.75
>       192         2    4.639E-06    9.159E-09      1.67      0.75
>       193         2    4.074E-06    9.159E-09      1.67      0.75
>       194         2    5.320E-06    9.159E-09      1.67      0.75
>       195         2    4.672E-06    9.159E-09      1.67      0.74
>       196         2    6.101E-06    9.159E-09      1.67      0.75
>       197         2    5.358E-06    9.159E-09      1.67      0.75
>       198         2    6.996E-06    9.159E-09      1.67      0.76
>       199         2    6.144E-06    9.159E-09      1.67      0.75
>       200         2    8.023E-06    9.159E-09      1.67      0.75
> 
>  EIGENVALUES(EV) AND OCCUPATION:
>      1    -11.2781946     2.000        2      0.7058206     2.000
>      3      0.7065389NC   2.000
>  CHEMICAL POTENTIAL =                             0.7065371502 EV
> 
>  TOTAL INTEGRATED ELECTRONIC DENSITY
>     IN G-SPACE =                                         6.049092
>     IN R-SPACE =                                         6.049092
> 
> 
>  VANDERBILT AUGMENTATION CHARGES (MEAN VALUE PER ATOM)
>  ATOM TYPE    NR. OF ATOMS        CHARGE
>        O           1               0.049
> 
>  (B+E2+X-V)             TOTAL ENERGY =          -16.81175790 A.U.
>  (B)                     BAND ENERGY =           -0.72510914 A.U.
>  (E2=I-H-S+R)   ELECTROSTATIC ENERGY =          -17.33584728 A.U.
>  (S)                           ESELF =           11.96826841 A.U.
>  (R)                             ESR =            0.00000000 A.U.
>  (X)     EXCHANGE-CORRELATION ENERGY =           -3.99099801 A.U.
>  (V)     EXCHANGE-CORRELATION POTEN. =           -5.24019667 A.U.
> 
>  ==------------------------------------------------------------==
>  ==     NFI=      1      ETOT=    -16.811758   TCPU=    173.96 ==
>  == DRHOMAX= 1.407E-01  DETOT=     0.000E+00    THL= 0.000E+00 ==
>  ==------------------------------------------------------------==
> 
>  RESTART INFORMATION WRITTEN ON FILE                  ./RESTART.1
>  ***    RWFOPT| THE NEW SIZE OF THE PROGRAM IS   75640/  95644 kBYTES ***
> 
>  ****************************************************************
>  *                                                              *
>  *                        FINAL RESULTS                         *
>  *                                                              *
>  ****************************************************************
> 
>  ****************************************************************
>  *                      ATOMIC COORDINATES                      *
>  ****************************************************************
>        1       O           7.558904       7.558904       7.558904
>  ****************************************************************
> 
> 
>  EIGENVALUES(EV) AND OCCUPATION:
>      1    -11.2781946     2.000        2      0.7058206     2.000
>      3      0.7065389NC   2.000
>  CHEMICAL POTENTIAL =                             0.7065371502 EV
> 
>  ****************************************************************
> 
> 
>  ELECTRONIC GRADIENT:
>     MAX. COMPONENT =    1.40719E-01         NORM =    6.04874E+00
> 
>  TOTAL INTEGRATED ELECTRONIC DENSITY
>     IN G-SPACE =                                         6.049092
>     IN R-SPACE =                                         6.049092
> 
> 
>  VANDERBILT AUGMENTATION CHARGES (MEAN VALUE PER ATOM)
>  ATOM TYPE    NR. OF ATOMS        CHARGE
>        O           1               0.049
> 
>  (B+E2+X-V)             TOTAL ENERGY =          -16.81175790 A.U.
>  (B)                     BAND ENERGY =           -0.72510914 A.U.
>  (E2=I-H-S+R)   ELECTROSTATIC ENERGY =          -17.33584728 A.U.
>  (S)                           ESELF =           11.96826841 A.U.
>  (R)                             ESR =            0.00000000 A.U.
>  (X)     EXCHANGE-CORRELATION ENERGY =           -3.99099801 A.U.
>  (V)     EXCHANGE-CORRELATION POTEN. =           -5.24019667 A.U.
> 
>  ****************************************************************
> 
> 
>  ================================================================
>                       BIG MEMORY ALLOCATIONS
>  SCR              1576657                PSI              1556068
>  QRL               903600                YLMB              856440
>  YF                778034                XF                778034
>  SCR               613400                PME               429264
>  RHOE              389017                HGPOT             389017
>  ----------------------------------------------------------------
>  [PEAK NUMBER   92]      PEAK MEMORY      9571930 =   76.6 MBytes
>  ================================================================
> 
> 
>  ****************************************************************
>  *                                                              *
>  *                            TIMING                            *
>  *                                                              *
>  ****************************************************************
>  SUBROUTINE            CALLS         CPU TIME        ELAPSED TIME
>     FFT-G/S             4372            39.07               38.96
>        VPSI             1002            37.95               38.13
>     S_FWFFT             1091            37.65               37.75
>    S_INVFFT             1095            36.25               38.53
>       QINIT                1            10.51               10.51
>     FNONLOC             1002             8.31                8.30
>        SPSI             1001             5.24                5.17
>      RNLSM1             1006             3.48                3.46
>    FRIESNER                1             2.61                2.65
>     VDBINIT                1             1.54                1.54
>        RHOV                2             1.08                1.09
>         HIP                2             1.06                1.08
>        NEWD                2             1.01                1.01
>        HPSI             1001             0.80                0.80
>       ATRHO                1             0.62                0.63
>     HOCKNEY                1             0.60                0.63
>       FWFFT                8             0.47                0.46
>  ----------------------------------------------------------------
>  TOTAL TIME                            188.25              190.71
>  ****************************************************************
> 
>        CPU TIME :    0 HOURS  3 MINUTES 10.52 SECONDS
>    ELAPSED TIME :    0 HOURS  3 MINUTES 13.71 SECONDS
> 
>  PROGRAM CPMD ENDED AT:   Fri Sep 17 00:49:35 2004
> 
> 3) KS energies with empty states
> 
> &CPMD
>   RESTART DENSITY
>   KOHN-SHAM ENERGIES
>    2
>   MAXSTEP
>   150
>   CENTER MOLECULE ON
> &END
> 
> 
> &DFT
>   NEWCODE
>   FUNCTIONAL LDA
>   LDA CORRELATION PZ
>   SLATER
>     0.666667
>   GC-CUTOFF
>   0.1E-07
> &END
> 
> &SYSTEM
>   SYMMETRY
>   0
>   ANGSTROM
>   CELL
>     8.0  1.0  1.0  0  0  0
>   CUTOFF SPHERICAL
>     55.0
> &END
> 
> &ATOMS
> *O_VDB_LDA.psp FORMATTED
>    LMAX=D LOC=D
>    1
>     0.000000    0.000000    0.000000
> &END
>  PROGRAM CPMD STARTED AT: Fri Sep 17 00:51:40 2004
> 
> 
> 
>                ******  ******    ****  ****  ******
>               *******  *******   **********  *******
>              ***       **   ***  ** **** **  **   ***
>              **        **   ***  **  **  **  **    **
>              **        *******   **      **  **    **
>              ***       ******    **      **  **   ***
>               *******  **        **      **  *******
>                ******  **        **      **  ******
> 
>                           VERSION 3.9.1
> 
>                             COPYRIGHT
>                       IBM RESEARCH DIVISION
>                 MPI FESTKOERPERFORSCHUNG STUTTGART
> 
>                        The CPMD consortium
>                     WWW:   http://www.cpmd.org
>                  Mailinglist:   cpmd-list at cpmd.org
>                      E-mail:   cpmd at cpmd.org
> 
> 
>                   ***  Aug 13 2004 -- 13:52:08  ***
> 
>  THE INPUT FILE IS:                                      o.inp-ks
>  THIS JOB RUNS ON:
>  THE CURRENT DIRECTORY IS:
>                                             /home/eariel/mycpmd/O
>  THE TEMPORARY DIRECTORY IS:
>                                             /home/eariel/mycpmd/O
>  THE PROCESS ID IS:                                          2546
>  THE JOB WAS SUBMITTED BY:                                 eariel
> 
> 
>  SINGLE POINT DENSITY OPTIMIZATION
> 
> 
>  EXACT DIAGONALIZATION OF KOHN-SHAM MATRIX
> 
>  PATH TO THE RESTART FILES:                                    ./
>  RESTART WITH OLD DENSITY
>  GRAM-SCHMIDT ORTHOGONALIZATION
>  MAXIMUM NUMBER OF STEPS:                                 1 STEPS
>  MAXIMUM NUMBER OF ITERATIONS FOR SC:                     1 STEPS
>  PRINT INTERMEDIATE RESULTS EVERY                     10001 STEPS
>  STORE INTERMEDIATE RESULTS EVERY                     10001 STEPS
>  STORE ELECTRONIC DENSITY IN RESTART FILE
>  NUMBER OF DISTINCT RESTART FILES:                              1
>  TEMPERATURE IS CALCULATED ASSUMING EXTENDED BULK BEHAVIOR
>  TIME STEP FOR ELECTRONS:                                  5.0000
>  TIME STEP FOR IONS:                                       5.0000
>  CONVERGENCE CRITERIA FOR WAVEFUNCTION OPTIMIZATION:   1.0000E-03
>  LANCZOS DIAGONALIZATION (KRYLOV SUBSPACE)
>     MAX. FRIESNER ITERATIONS                                  200
>     MAX. KRYLOV SUBSPACE                                        6
>     MAX. KRYLOV BLOCK SIZE       FIXED LATER (WAITING FOR NSTATE)
>     MAX. BETA^2                                        1.0000E-08
>  ANDERSON MIXING PARAMETER:                            2.0000E-01
>  BROYDEN MIXING PARAMETER [BROYMIX]                    1.5000E-01
>  BROYDEN CUTOFF [ECUTBROY]            EQUAL TO THE DENSITY CUTOFF
>  BROYDEN MIXING STARTS [NFRBROY] AFTER                    0 STEPS
>  BROYDEN MIXING RESET [IBRESET] AFTER                     8 STEPS
>  BROYDEN MIXING W02                                    1.0000E-02
>  ALEXANDER MIXING:                                         0.9000
>  SPLINE INTERPOLATION IN G-SPACE FOR PSEUDOPOTENTIAL FUNCTIONS
>     NUMBER OF SPLINE POINTS:                                 5000
> 
>  EXCHANGE CORRELATION FUNCTIONALS
>     LDA EXCHANGE:                        SLATER (ALPHA = 0.66667)
>     LDA CORRELATION:                              PERDEW & ZUNGER
>        [J.P. PERDEW AND A ZUNGER, PRB 23 5048 (1981)]
> 
>  ***     DETSP| THE NEW SIZE OF THE PROGRAM IS    1940/  22060 kBYTES ***
> 
>  >>>>>>>> CENTER OF MASS HAS BEEN MOVED TO CENTER OF BOX <<<<<<<<
> 
> 
>  ***************************** ATOMS ****************************
>    NR   TYPE        X(bohr)        Y(bohr)        Z(bohr)     MBL
>     1      O       7.558904       7.558904       7.558904       3
>  ****************************************************************
> 
>  NUMBER OF STATES:                                              5
>  NUMBER OF ELECTRONS:                                     6.00000
>  CHARGE:                                                  0.00000
>  ELECTRON TEMPERATURE(KELVIN):                            0.00000
>  OCCUPATION
>   2.0  2.0  2.0  0.0  0.0
> 
>  LANCZOS DIAGONALIZATION (KRYLOV SUBSPACE)
>     MAX. KRYLOV BLOCK SIZE                                      5
> 
>    ============================================================
>    |  pseudopotential report: version  7.3.4 date  6-12-2003  |
>    ------------------------------------------------------------
>    |  oxygen                    ceperley-alder exchange-corr  |
>    |  z =   8.00  zv =   6.00  exfact =   0.00000             |
>    |                            etot  = -31.51046             |
>    |  index    orbital      occupation    energy              |
>    |    1        200           2.00       -1.74               |
>    |    2        210           4.00       -0.68               |
>    |  keyps = 3     ifpcor = 0                                |
>    |  rinner =      0.80     for L=    1                      |
>    |  rinner =      0.80     for L=    2                      |
>    |  rinner =      0.80     for L=    3                      |
>    |    new generation scheme:                                |
>    |    nbeta =  4     kkbeta =  507     rcloc =    1.0000    |
>    |    ibeta     l     epsilon   rcut iptype                 |
>    |       1      0      -1.74   1.10      2                  |
>    |       2      0      -0.20   1.10      2                  |
>    |       3      1      -0.80   1.10      2                  |
>    |       4      1       0.20   1.10      2                  |
>    |  npf    = 8  ptryc =  10.000                             |
>    |  lloc   = 2  eloc   =   0.000                            |
>    |  ifqopt = 2  nqf    = 8  qtryc =  10.000                 |
>    |  all electron calculation used schroedinger equation     |
>    |         ************logarithmic mesh************         |
>    ============================================================
> 
>  ****************************************************************
>  *   ATOM       MASS   RAGGIO NLCC              PSEUDOPOTENTIAL *
>  *     O     15.9994   1.2000   NO              VANDERBILT      *
>  ****************************************************************
> 
> 
>  OPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPEN
>  NUMBER OF CPUS PER TASK                                        1
>  OPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPENMPOPEN
> 
>  ***     RGGEN| THE NEW SIZE OF THE PROGRAM IS    8656/  36592 kBYTES ***
> 
>  ************************** SUPERCELL ***************************
>  THIS IS AN ISOLATED SYSTEM CALCULATION
>  POISSON EQUATION SOLVER  :                               HOCKNEY
>  COULOMB SMOOTHING RADIUS :                                 1.080
>  SYMMETRY:                                           SIMPLE CUBIC
>  LATTICE CONSTANT(a.u.):                                 15.11781
>  CELL DIMENSION:  15.1178  1.0000  1.0000  0.0000  0.0000  0.0000
>  VOLUME(OMEGA IN BOHR^3):                              3455.14651
>  LATTICE VECTOR A1(BOHR):           15.1178     0.0000     0.0000
>  LATTICE VECTOR A2(BOHR):            0.0000    15.1178     0.0000
>  LATTICE VECTOR A3(BOHR):            0.0000     0.0000    15.1178
>  RECIP. LAT. VEC. B1(2Pi/BOHR):      0.0661     0.0000     0.0000
>  RECIP. LAT. VEC. B2(2Pi/BOHR):      0.0000     0.0661     0.0000
>  RECIP. LAT. VEC. B3(2Pi/BOHR):      0.0000     0.0000     0.0661
>  REAL SPACE MESH:                    72           72           72
>  WAVEFUNCTION CUTOFF(RYDBERG):                           55.00000
>  DENSITY CUTOFF(RYDBERG):          (DUAL= 4.00)         220.00000
>  NUMBER OF PLANE WAVES FOR WAVEFUNCTION CUTOFF:             11924
>  NUMBER OF PLANE WAVES FOR DENSITY CUTOFF:                  95160
>  NUMBER OF PLANE WAVES FOR BROYDEN MIXING:                  95160
>  ****************************************************************
> 
>  ***  RINFORCE| THE NEW SIZE OF THE PROGRAM IS   19336/  48876 kBYTES ***
>  ***    FFTPRP| THE NEW SIZE OF THE PROGRAM IS   30400/  50196 kBYTES ***
>  ***   CLUSTER| THE NEW SIZE OF THE PROGRAM IS   34304/  53980 kBYTES ***
> 
>  GENERATE ATOMIC BASIS SET
>       O        SLATER ORBITALS
>         2S        ALPHA=   2.2458      OCCUPATION= 2.00
>         2P        ALPHA=   2.2266      OCCUPATION= 4.00
> 
> 
>  INITIALIZATION TIME:                               13.06 SECONDS
> 
>  ***    WFOPTS| THE NEW SIZE OF THE PROGRAM IS   34520/  63288 kBYTES ***
>  RV30! NUMBER OF STATES   HAS CHANGED                      3    5
>  RV30| WARNING! NO DENSITY INFORMATION
> 
>  RESTART INFORMATION READ ON FILE                       ./RESTART
>  ***     PHFAC| THE NEW SIZE OF THE PROGRAM IS   34780/  92592 kBYTES ***
>  ***    ATOMWF| THE NEW SIZE OF THE PROGRAM IS   34984/  94088 kBYTES ***
>   ATRHO| WARNING! THE NUMBER OF GENERATED ATOMIC STATE (4)
>   ATRHO| WARNING! IS LESS THAN THE NUMBER OF STATE (5)
>   ATRHO| WARNING!     1 STATES ARE EQUAL TO ZERO
>   ATRHO| USE SECTION BASIS TO SPECIFY ATOMIC BASIS
>   ATRHO| CHARGE(R-SPACE):    6.000000      (G-SPACE):    6.000000
>  ATOMWF| WARNING! RANDOMIZATION OF     1 STATES
> 
>  ****************************************************************
>  *                      ATOMIC COORDINATES                      *
>  ****************************************************************
>        1       O           7.558904       7.558904       7.558904
>  ****************************************************************
> 
>   !! WARNING FROM DETDOF: WHY IS GLIB LESS THAN UNITY !!
>   !! WARNING FROM DETDOF: NOW IT IS SET EQUAL TO UNITY !!
> 
>  DEGREES OF FREEDOM FOR SYSTEM:                                 1
> 
>  CPU TIME FOR WAVEFUNCTION INITIALIZATION:           3.41 SECONDS
>  ***    RWFOPT| THE NEW SIZE OF THE PROGRAM IS   65308/  92728 kBYTES ***
>   EWALD| SUM IN REAL SPACE OVER                     1* 1* 1 CELLS
> 
>  <<<<<<<<<<<<<<<<<<< LANCZOS DIAGONALIZATION <<<<<<<<<<<<<<<<<<<<
>  >> TIME FOR INITIAL SUBSPACE DIAGONALIZATION:               0.49
>  >> CYCLE     NCONV        B2MAX        B2MIN     #HPSI      TIME
>         1         0    1.561E-01    4.181E-02      6.00      2.38
>         2         0    1.563E-01    5.488E-03      5.00      2.39
>         3         0    6.679E-02    2.159E-03      5.00      2.40
>         4         0    5.013E-02    7.902E-04      5.00      2.39
>         5         0    2.733E-02    3.050E-04      5.00      2.40
>         6         0    2.384E-02    9.732E-05      5.00      2.40
>         7         0    1.440E-02    3.847E-05      5.00      2.39
>         8         0    1.341E-02    1.197E-05      5.00      2.39
>         9         0    8.518E-03    5.429E-06      5.00      2.40
>        10         0    8.238E-03    1.632E-06      5.00      2.39
>        11         0    5.415E-03    8.208E-07      5.00      2.40
>        12         0    5.396E-03    2.484E-07      5.00      2.39
>        13         0    3.645E-03    1.290E-07      5.00      2.40
>        14         0    3.716E-03    3.949E-08      5.00      2.39
>        15         0    2.562E-03    2.070E-08      5.00      2.39
>        16         1    2.657E-03    8.884E-09      4.40      1.96
>        17         1    1.860E-03    8.884E-09      4.00      1.65
>        18         1    1.952E-03    8.884E-09      4.00      1.66
>        19         1    1.380E-03    8.884E-09      4.00      1.65
>        20         1    1.460E-03    8.884E-09      4.00      1.65
>        21         1    1.040E-03    8.884E-09      4.00      1.66
>        22         1    1.106E-03    8.884E-09      4.00      1.65
>        23         1    7.907E-04    8.884E-09      4.00      1.65
>        24         1    8.436E-04    8.884E-09      4.00      1.65
>        25         1    6.049E-04    8.884E-09      4.00      1.66
>        26         1    6.467E-04    8.884E-09      4.00      1.65
>        27         1    4.645E-04    8.884E-09      4.00      1.65
>        28         1    4.972E-04    8.884E-09      4.00      1.65
>        29         1    3.575E-04    8.884E-09      4.00      1.66
>        30         1    3.830E-04    8.884E-09      4.00      1.65
>        31         1    2.755E-04    8.884E-09      4.00      1.65
>        32         1    2.953E-04    8.884E-09      4.00      1.66
>        33         1    2.125E-04    8.884E-09      4.00      1.65
>        34         1    2.278E-04    8.884E-09      4.00      1.65
>        35         1    1.640E-04    8.884E-09      4.00      1.65
>        36         1    1.758E-04    8.884E-09      4.00      1.66
>        37         1    1.265E-04    8.884E-09      4.00      1.65
>        38         1    1.356E-04    8.884E-09      4.00      1.65
>        39         1    9.766E-05    8.884E-09      4.00      1.65
>        40         1    1.047E-04    8.884E-09      4.00      1.66
>        41         1    7.538E-05    8.884E-09      4.00      1.65
>        42         1    8.081E-05    8.884E-09      4.00      1.65
>        43         1    5.818E-05    8.884E-09      4.00      1.66
>        44         1    6.237E-05    8.884E-09      4.00      1.65
>        45         1    4.491E-05    8.884E-09      4.00      1.65
>        46         1    4.814E-05    8.884E-09      4.00      1.65
>        47         1    3.466E-05    8.884E-09      4.00      1.66
>        48         1    3.716E-05    8.884E-09      4.00      1.65
>        49         1    2.675E-05    8.884E-09      4.00      1.65
>        50         2    2.868E-05    8.884E-09      3.80      1.64
>        51         2    2.065E-05    8.884E-09      3.00      1.58
>        52         2    2.214E-05    8.884E-09      3.00      1.57
>        53         2    1.594E-05    8.884E-09      3.00      1.57
>        54         2    1.709E-05    8.884E-09      3.00      1.58
>        55         2    1.230E-05    8.884E-09      3.00      1.57
>        56         2    1.319E-05    8.884E-09      3.00      1.57
>        57         2    9.497E-06    8.884E-09      3.00      1.57
>        58         2    1.018E-05    8.884E-09      3.00      1.58
>        59         2    7.330E-06    8.884E-09      3.00      1.57
>        60         2    7.860E-06    8.884E-09      3.00      1.58
>        61         2    5.658E-06    8.884E-09      3.00      1.57
>        62         2    6.067E-06    8.884E-09      3.00      1.58
>        63         2    4.368E-06    8.884E-09      3.00      1.57
>        64         2    4.684E-06    8.884E-09      3.00      1.58
>        65         2    3.372E-06    8.884E-09      3.00      1.57
>        66         2    3.616E-06    8.884E-09      3.00      1.57
>        67         2    2.603E-06    8.884E-09      3.00      1.57
>        68         2    2.791E-06    8.884E-09      3.00      1.57
>        69         2    2.009E-06    8.884E-09      3.00      1.58
>        70         2    2.155E-06    8.884E-09      3.00      1.57
>        71         2    1.551E-06    8.884E-09      3.00      1.57
>        72         2    1.664E-06    8.884E-09      3.00      1.57
>        73         2    1.198E-06    8.884E-09      3.00      1.58
>        74         2    1.284E-06    8.884E-09      3.00      1.57
>        75         2    9.245E-07    8.884E-09      3.00      1.58
>        76         3    9.915E-07    8.884E-09      2.40      1.13
>        77         3    7.137E-07    8.884E-09      2.00      0.83
>        78         3    7.655E-07    8.884E-09      2.00      0.84
>        79         3    5.511E-07    8.884E-09      2.00      0.83
>        80         3    5.910E-07    8.884E-09      2.00      0.83
>        81         3    4.254E-07    8.884E-09      2.00      0.83
>        82         3    4.563E-07    8.884E-09      2.00      0.83
>        83         3    3.285E-07    8.884E-09      2.00      0.84
>        84         3    3.523E-07    8.884E-09      2.00      0.83
>        85         3    2.536E-07    8.884E-09      2.00      0.83
>        86         3    2.721E-07    8.884E-09      2.00      0.84
>        87         3    1.958E-07    8.884E-09      2.00      0.83
>        88         3    2.101E-07    8.884E-09      2.00      0.83
>        89         3    1.512E-07    8.884E-09      2.00      0.84
>        90         3    1.622E-07    8.884E-09      2.00      0.83
>        91         3    1.167E-07    8.884E-09      2.00      0.84
>        92         3    1.252E-07    8.884E-09      2.00      0.83
>        93         3    9.014E-08    8.884E-09      2.00      0.83
>        94         3    9.671E-08    8.884E-09      2.00      0.84
>        95         3    6.960E-08    8.884E-09      2.00      0.83
>        96         3    7.468E-08    8.884E-09      2.00      0.84
>        97         3    5.374E-08    8.884E-09      2.00      0.83
>        98         3    5.766E-08    8.884E-09      2.00      0.83
>        99         3    4.150E-08    8.884E-09      2.00      0.84
>       100         3    4.453E-08    8.884E-09      2.00      0.83
>       101         3    3.204E-08    8.884E-09      2.00      0.83
>       102         3    3.439E-08    8.884E-09      2.00      0.84
>       103         3    2.474E-08    8.884E-09      2.00      0.84
>       104         3    2.655E-08    8.884E-09      2.00      0.83
>       105         3    1.911E-08    8.884E-09      2.00      0.83
>       106         3    2.050E-08    8.884E-09      2.00      0.83
>       107         5    9.530E-09    8.884E-09      0.80      0.35
> 
>  EIGENVALUES(EV) AND OCCUPATION:
>      1    -11.2781946     2.000        2     -0.3815193     2.000
>      3     -0.2300328     2.000        4      0.7065208     0.000
>      5      0.7065390     0.000
>  CHEMICAL POTENTIAL =                            -0.2300326449 EV
> 
>  TOTAL INTEGRATED ELECTRONIC DENSITY
>     IN G-SPACE =                                         6.034344
>     IN R-SPACE =                                         6.034344
> 
> 
>  VANDERBILT AUGMENTATION CHARGES (MEAN VALUE PER ATOM)
>  ATOM TYPE    NR. OF ATOMS        CHARGE
>        O           1               0.034
> 
>  (B+E2+X-V)             TOTAL ENERGY =          -16.96050918 A.U.
>  (B)                     BAND ENERGY =           -0.87386055 A.U.
>  (E2=I-H-S+R)   ELECTROSTATIC ENERGY =          -17.33584728 A.U.
>  (S)                           ESELF =           11.96826841 A.U.
>  (R)                             ESR =            0.00000000 A.U.
>  (X)     EXCHANGE-CORRELATION ENERGY =           -3.99099801 A.U.
>  (V)     EXCHANGE-CORRELATION POTEN. =           -5.24019667 A.U.
> 
>  ==------------------------------------------------------------==
>  ==     NFI=      1      ETOT=    -16.960509   TCPU=    162.84 ==
>  == DRHOMAX= 1.439E-01  DETOT=     0.000E+00    THL= 0.000E+00 ==
>  ==------------------------------------------------------------==
> 
>  RESTART INFORMATION WRITTEN ON FILE                  ./RESTART.1
>  ***    RWFOPT| THE NEW SIZE OF THE PROGRAM IS   78992/  98804 kBYTES ***
> 
>  ****************************************************************
>  *                                                              *
>  *                        FINAL RESULTS                         *
>  *                                                              *
>  ****************************************************************
> 
>  ****************************************************************
>  *                      ATOMIC COORDINATES                      *
>  ****************************************************************
>        1       O           7.558904       7.558904       7.558904
>  ****************************************************************
> 
> 
>  EIGENVALUES(EV) AND OCCUPATION:
>      1    -11.2781946     2.000        2     -0.3815193     2.000
>      3     -0.2300328     2.000        4      0.7065208     0.000
>      5      0.7065390     0.000
>  CHEMICAL POTENTIAL =                            -0.2300326449 EV
> 
>  ****************************************************************
> 
> 
>  ELECTRONIC GRADIENT:
>     MAX. COMPONENT =    1.43915E-01         NORM =    6.89928E+00
> 
>  TOTAL INTEGRATED ELECTRONIC DENSITY
>     IN G-SPACE =                                         6.034344
>     IN R-SPACE =                                         6.034344
> 
> 
>  VANDERBILT AUGMENTATION CHARGES (MEAN VALUE PER ATOM)
>  ATOM TYPE    NR. OF ATOMS        CHARGE
>        O           1               0.034
> 
>  (B+E2+X-V)             TOTAL ENERGY =          -16.96050918 A.U.
>  (B)                     BAND ENERGY =           -0.87386055 A.U.
>  (E2=I-H-S+R)   ELECTROSTATIC ENERGY =          -17.33584728 A.U.
>  (S)                           ESELF =           11.96826841 A.U.
>  (R)                             ESR =            0.00000000 A.U.
>  (X)     EXCHANGE-CORRELATION ENERGY =           -3.99099801 A.U.
>  (V)     EXCHANGE-CORRELATION POTEN. =           -5.24019667 A.U.
> 
>  ****************************************************************
> 
> 
>  ================================================================
>                       BIG MEMORY ALLOCATIONS
>  SCR              1576657                PSI              1556068
>  QRL               903600                YLMB              856440
>  YF                778034                XF                778034
>  PME               715440                SCR               613400
>  RHOE              389017                HGPOT             389017
>  ----------------------------------------------------------------
>  [PEAK NUMBER   92]      PEAK MEMORY      9977414 =   79.8 MBytes
>  ================================================================
> 
> 
>  ****************************************************************
>  *                                                              *
>  *                            TIMING                            *
>  *                                                              *
>  ****************************************************************
>  SUBROUTINE            CALLS         CPU TIME        ELAPSED TIME
>     FFT-G/S             3972            35.52               35.46
>        VPSI              534            33.82               33.85
>     S_FWFFT              991            33.41               33.52
>    S_INVFFT              995            32.97               32.92
>     FNONLOC              534            11.30               11.34
>       QINIT                1            10.55               10.55
>        SPSI              533             5.33                5.38
>      RNLSM1              538             3.45                3.43
>    FRIESNER                1             3.23                3.24
>     VDBINIT                1             1.41                1.41
>        RHOV                2             1.08                1.07
>        HPSI              533             1.03                1.01
>         HIP                2             1.02                1.03
>        NEWD                2             0.98                0.98
>     HOCKNEY                1             0.66                0.67
>       ATRHO                1             0.57                0.59
>       FWFFT                8             0.45                0.46
>      OVLAP2              110             0.45                0.42
>      INVFFT                7             0.40                0.40
>  ----------------------------------------------------------------
>  TOTAL TIME                            177.63              177.74
>  ****************************************************************
> 
>        CPU TIME :    0 HOURS  2 MINUTES 59.40 SECONDS
>    ELAPSED TIME :    0 HOURS  3 MINUTES  1.25 SECONDS
> 
>  PROGRAM CPMD ENDED AT:   Fri Sep 17 00:54:41 2004
> 
> Other options that I have tried:
> 
> &CPMD
>   OPTIMIZE WAVEFUNCTION
>   #  PCG MINIMIZE
>   #  TIMESTEP
>   #   5
>   RESTART ALL
>   LANCZOS DIAGONALISATION ALL
> 
>   &DFT
>   GC-CUTOFF
>     0.1E-05  # Sugeted for ultrasoft PP
> 
>  POISSON SOLVER TUCKERMAN
> 
> What is wrong?
> 
> Thank you
> 
> Eduardo A. Menendez Proupin
> Department of Physics
> Faculty of Science
> University of Chile
> Las Palmeras 3425
> Ñuñoa, Santiago
> Chile
> Phone: 56+2+678 74 11
> http://fisica.ciencias.uchile.cl/~emenendez/
> 
> _______________________________________________
> CPMD-list mailing list
> CPMD-list at cpmd.org
> http://cpmd.org/mailman/listinfo/cpmd-list
> 



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