[CPMD-list] Torsion constraints

Ari P Seitsonen Ari.P.Seitsonen at iki.fi
Mon Apr 26 22:43:22 CEST 2004


Dear Erik,

  There's indeed a bug in the CPMD version 3.7.*, and it's exactly the 
phase of the angle (-1 degree becomes 359 or vice versa). It should be 
fixed in the new version (out any day now...!! I hope). Sorry for the 
inconvenience.

  GNMAX is the largest simple component of ionic forces, however 
what's printed with the coordinates are the forces without/before the 
applying the constraints, that's why GNMAX is huge even though the forces 
in the output seem to be small.

    Greetings,

       apsi

-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-=*=-
 Ari Paavo Seitsonen / Ari.P.Seitsonen at iki.fi / http://www.iki.fi/~apsi/
 Tel +41 1 635 44 97 / Fax +41 1 635 68 38 / GSM +41 79 719 09 35      
 Anschrift: Physikalisch Chemisches Institut (PCI), Universität Zürich (UniZh)
 Indirizzo: Winterthurerstraße 190, CH-8057 Zürich
 Address:   Schweiz / Svizzera / Suisse / Svizra / Switzerland

On Sun, 18 Apr 2004, Erik Santiso wrote:

> Hi,
> 
> I've been doing some geometry optimizations with torsion constraints, and
> for most cases thinks seem to work well. However, if I set a torsion angle
> to be 0 degrees (or 360), the geometry optimization starts doing funny
> things. Here's an example. The constraint in this case is that the torsion
> between atoms 7, 8, 9, 10 should be 0.0:
> 
>    ATOM          COORDINATES            GRADIENTS (-FORCES)
>    1  H  0.6369 11.2421  7.3588   0.132E-03 -0.197E-04  0.250E-03
>    2  H  2.7954 13.9975  7.3282  -0.144E-03  0.423E-04 -0.288E-03
>    3  H -3.0319 13.9637  7.3442   0.110E-03  0.155E-04 -0.891E-04
>    4  H -3.0301 18.4817  7.3516  -0.723E-04  0.549E-04  0.348E-03
>    5  H  0.6320 21.2032  7.3462   0.238E-04 -0.108E-03 -0.193E-03
>    6  H  2.7974 18.4518  7.3616  -0.199E-04 -0.110E-03  0.265E-03
>    7  C  0.8615 13.2867  7.3435   0.171E-03 -0.140E-03  0.750E-03
>    8  C -1.1573 14.8298  7.3389  -0.341E-03  0.187E-03 -0.477E-03
>    9  C -1.1552 17.6146  7.3452   0.332E-03 -0.267E-03  0.557E-03
>   10  C  0.8619 19.1595  7.3501  -0.956E-05  0.325E-03  0.346E-03
>  ****************************************************************
>  *** TOTAL STEP NR.   166           GEOMETRY STEP NR.     24  ***
>  *** GNMAX=  1.696295E-02 [8.02E-03]     ETOT=    -26.304652  ***
>  *** GNORM=  4.848471E-03               DETOT=    -1.048E-05  ***
>  *** CNSTR=  1.745681E-02                TCPU=         31.09  ***
>  ****************************************************************
>    1  2.674E-04   4.708E-05     -26.304543    1.082E-04      4.04
>    2  1.048E-04   1.539E-05     -26.304644   -1.002E-04      4.07
>    3  5.823E-05   8.073E-06     -26.304651   -7.269E-06      4.05
>    4  5.257E-05   4.483E-06     -26.304654   -3.038E-06      4.10
>    5  2.776E-05   2.903E-06     -26.304654   -6.502E-07      4.10
>    6  1.711E-05   1.621E-06     -26.304655   -4.005E-07      4.90
>    7  1.186E-05   6.911E-07     -26.304655   -2.197E-07      4.78
>    8  6.332E-06   3.436E-07     -26.304655   -6.332E-09      4.85
> 
>  RESTART INFORMATION WRITTEN ON FILE                  ./RESTART.1
> 
>    ATOM          COORDINATES            GRADIENTS (-FORCES)
>    1  H  0.6355 11.2413  7.3588   0.526E-04 -0.877E-04  0.409E-03
>    2  H  2.7954 13.9970  7.3292  -0.168E-03  0.962E-04 -0.229E-04
>    3  H -3.0314 13.9634  7.3479   0.132E-03 -0.633E-05 -0.574E-04
>    4  H -3.0297 18.4816  7.3509  -0.160E-03  0.100E-03  0.300E-03
>    5  H  0.6309 21.2036  7.3458   0.320E-04 -0.158E-03 -0.187E-03
>    6  H  2.7984 18.4542  7.3634   0.473E-04 -0.805E-04  0.287E-03
>    7  C  0.8617 13.2859  7.3373   0.252E-03 -0.145E-03  0.562E-04
>    8  C -1.1569 14.8295  7.3402  -0.414E-03  0.118E-03 -0.197E-03
>    9  C -1.1545 17.6146  7.3461   0.506E-03 -0.255E-03  0.583E-03
>   10  C  0.8621 19.1602  7.3504  -0.729E-04  0.368E-03  0.278E-03
>  ****************************************************************
>  *** TOTAL STEP NR.   174           GEOMETRY STEP NR.     25  ***
>  *** GNMAX=  3.285935E+01 [6.14E-03]     ETOT=    -26.304655  ***
>  *** GNORM=  9.384478E+00               DETOT=    -3.556E-06  ***
>  *** CNSTR=  3.285993E+01                TCPU=         34.97  ***
>  ****************************************************************
>    1  2.379E-04   4.148E-05     -26.304568    8.690E-05      4.05
>    2  9.553E-05   1.362E-05     -26.304642   -7.339E-05      4.02
>    3  5.412E-05   7.187E-06     -26.304650   -8.253E-06      4.04
>    4  4.862E-05   3.975E-06     -26.304651   -1.259E-06      4.21
>    5  2.584E-05   2.507E-06     -26.304652   -7.716E-07      4.10
>    6  1.562E-05   1.417E-06     -26.304652   -3.099E-07      4.83
>    7  1.029E-05   5.705E-07     -26.304652   -7.033E-08      4.83
>    8  5.174E-06   2.462E-07     -26.304652   -3.037E-08      4.79
> 
>  RESTART INFORMATION WRITTEN ON FILE                  ./RESTART.1
> 
>    ATOM          COORDINATES            GRADIENTS (-FORCES)
>    1  H  0.6367 11.2421  7.3587   0.158E-03  0.159E-04  0.284E-03
>    2  H  2.7959 13.9965  7.3279  -0.479E-04  0.339E-04 -0.247E-03
>    3  H -3.0317 13.9639  7.3445   0.308E-04  0.242E-04 -0.100E-03
>    4  H -3.0299 18.4821  7.3517   0.805E-04  0.338E-04  0.350E-03
>    5  H  0.6315 21.2030  7.3463   0.164E-04 -0.373E-04 -0.187E-03
>    6  H  2.7977 18.4529  7.3624  -0.468E-05 -0.183E-04  0.273E-03
>    7  C  0.8614 13.2866  7.3426  -0.168E-03 -0.316E-04  0.715E-03
>    8  C -1.1568 14.8297  7.3389   0.467E-04  0.347E-04 -0.483E-03
>    9  C -1.1557 17.6147  7.3453   0.256E-04 -0.184E-03  0.562E-03
>   10  C  0.8618 19.1591  7.3502   0.529E-04  0.812E-04  0.308E-03
>  ****************************************************************
>  *** TOTAL STEP NR.   182           GEOMETRY STEP NR.     26  ***
>  *** GNMAX=  1.532222E-02 [5.30E-03]     ETOT=    -26.304652  ***
>  *** GNORM=  4.377040E-03               DETOT=     2.814E-06  ***
>  *** CNSTR=  1.581241E-02                TCPU=         34.95  ***
>  ****************************************************************
>    1  8.455E-06   2.055E-06     -26.304652    2.594E-07      4.12
>    2  6.064E-06   6.952E-07     -26.304652   -2.099E-07      4.85
> 
>  RESTART INFORMATION WRITTEN ON FILE                  ./RESTART.1
> 
> In the middle step (25), it appears that the constraint has a difference
> of 32.8, but the torsion angle is actually much smaller (the coordinates
> of the 4 atoms are pretty much equal to those in the other two steps). Any
> idea what is causing this? One thing that comes to mind is the
> discontinuity of the torsion angle at 0 (360), could this be the cause
> (and if it is, is there any way around it?).
> 
> I also have another question. What are exactly the quantities in the GNMAX
> line of the output at each geometry step? Before I thought it was the
> maximum nuclear gradient, but in this case it is clearly not.
> 
> Thanks a lot!
> 
> Erik.
> 
> -------------------------------------
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